Friday, January 11, 2019

Ligand-modulated ring-expansion

GA?id=C8CC09710K

Chem. Commun., 2019, Advance Article
DOI: 10.1039/C8CC09710K, Communication
Veronica Carta, Miguel A. Soto, Mark J. MacLachlan
An unstrained metal-containing macrocycle was ring-expanded by a ring-opening metathesis strategy, leading to the formation of a bimetallic dimeric macrocycle. The reaction is driven by coordination of a bulky ligand, 2,6-lutidine, on the fourth coordination site of the palladium center. In the absence of metal, or with a less bulky ligand, the ring-expansion reaction does not proceed.
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